Ronald Wyatt (segment 4 "The Man Who Collected Poe")
Jack Palance
Dr. Diabolo (Framing Story)
Burgess Meredith
Carla Hayes (segment 2 "Terror Over Hollywood")
Beverly Adams
Carla Hayes
Beverly Adams
Lancelot Canning (segment 4 "The Man Who Collected Poe")
Peter Cushing
Colin Williams (segment 1 "Enoch")
Michael Bryant
Dorothy Endicott (segment 3 "Mr. Steinway")
Barbara Ewing
Uncle Roger (segment 1 "Enoch")
Maurice Denham
Leo Winston (segment 3 "Mr. Steinway")
John Standing
Bruce Benton (segment 2 "Terror Over Hollywood")
Robert Hutton
Eddie Storm (segment 2 "Terror Over Hollywood")
John Phillips
Gordon Roberts (Framing Story)
Michael Ripper
Dr. Heim
Bernard Kay
Dr. Heim (segment 2 "Terror Over Hollywood")
Bernard Kay
Nurse Parker (segment 1 "Enoch")
Catherine Finn
Miss Maxine Chambers (segment 3 "Mr. Steinway")
Ursula Howells
Mike Charles (segment 2 "Terror Over Hollywood")
David Bauer
Dr. Silversmith (segment 1 "Enoch")
Niall MacGinnis
Fairground Barker
Timothy Bateson
Millie
Nicole Shelby
Atropos
Clytie Jessop
Constable
Michael Hawkins
Edgar Allan Poe
Hedger Wallace
Tramp
Frank Forsyth
Constable
Roy Stephens
Constable
Roy Stevens
Edgar Allan Poe
Geoffrey Wallace
Fred
James Copeland
Police Sergeant
Norman Claridge
Collector
Roy Goldfrey
Tramp
Barry Lowe
Tramp
Barry Low