Gargamel

Hank Azaria

Patrick Winslow

Neil Patrick Harris

Grace Winslow

Jayma Mays

Odile

Sofía Vergara

Henri

Tim Gunn

Papa Smurf (voice)

Jonathan Winters

Smurfette (voice)

Katy Perry

Clumsy Smurf (voice)

Anton Yelchin

Gutsy Smurf (voice)

Alan Cumming

Brainy Smurf (voice)

Fred Armisen

Grouchy Smurf (voice)

George Lopez

Jokey Smurf (voice)

Paul Reubens

Azrael (voice)

Frank Welker

Model

Madison McKinley

Model

Meg Phillips

Greedy

Kenan Thompson

Cabbie

Mahadeo Shivraj

Handy

Jeff Foxworthy

Newscaster

Julie Chang

Vanity

John Oliver

Chef

Wolfgang Puck

Bluetooth Businessman

Mark Doherty

Young Woman

Minglie Chen

Hefty Smurf (voice)

Gary Basaraba

Baker Smurf (voice)

B.J. Novak

Guy in Plaid Shirt

Sean Kenin

Narrator Smurf (voice)

Tom Kane

Bum

Victor Pagan

Anjelou Employee

Adria Baratta

Crazy Smurf (Voice)

John Kassir

Farmer Smurf (voice)

Joel McCrary

Odile's Mother

Paula Pizzi

Waiter

Andrew Sellon

Little Sister

Julianna Rigoglioso

Blonde Sister

Daria Rae Figlo

Toy Salesperson

Bradley Gosnell

Newscaster

Roger Clark

Toy Store Parent

Heidi Armbruster

Toy Store Parent

Finnerty Steeves

Parent with Girls

John Speredakos

Kicking Girl

Skai Jackson

Skateboard Kid

Alex Hall

Skateboard Kid

Eric Redgate

FAO Custodian

Jojo Gonzalez

Cop

Scott Dillin

Cop

Tyree Michael Simpson

Inmate Bubba

Sean Ringgold

Blonde Sister

Daria Rae Figlio

Bubba's Inmate Friend

Mario D'Leon

Party Guest

Liz Smith

Party Guest

Tom Colicchio

Party Guest

Michael Musto

Party Guest

Joan Rivers

Party Guest

Olivia Palermo

Party Guest

Julia Enescu

Party Guest

Lauren Waggoner

Azrael

Mr. Krinkle

Cop

Scotty Dillin

Elway

Hank

Party Guest

Julia T. Enescu

Mandy Patinkin

Philipp Moog

Stefan Staudinger

Cathlen Gawlich

Jeff Burrell

Iris Artajo

Thomas Nero Wolff